Before presenting the R&B singer with a Brit Award, Cole, 27, declared: "And the winner of the Best International Female solo artist is, my girl crush, what's her name? Rihanna."
Last year Rihanna revealed that she had a girl crush on Cole and at the time, the 22-year-old said of 'The X Factor' judge: "She is awesome, I think she is the most beautiful woman I have ever seen.
"Like, how do you have a face like that, with hair like that and dimples, and a body like that, that's proportioned like that."
Before receiving her Brit Award, Rihanna, real name Robyn Rihanna Fenty, performed a medley of tracks from her recent album 'Loud', despite complaining of feeling under the weather.
The Barbadian arrived at London's O2 Arena in a psychedelic Dior prom dress, costing in excess of €12k (10k), before changing twice as she took to the stage.
However she headed straight back to LA after collecting her award due to her illness - which she described as "the bug that's going around."
Girls Aloud star Cole missed out on a gong at the ceremony, she was nominated for Best British Female, which went to Laura Marling.
In an interview backstage with Dave Berry, Cole said of Rihanna: "I love her".
When asked if the feeling is mutual, she said: "Yeah, she loves us."
Then Cole was asked if there was any chance of a duet between the two singers and she said: "I'd love that, to do a single together, to do a record with her.
"She feels the same, there could be wheels, there could be motions."
When Berry suggested that Jay Z could be the mentor in the collaboration, Cole replied: "I hadn't thought of that but now you've put it in my head, that could be amazing."
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